HR: 14:25h
AN: A22D-04 [PDF]
TI: The Role of Atmospheric Organic Nitrogen in Forest Nitrogen Cycling
AU: * Lockwood, A
EM: manders1321@cs.com
AF: Department of Chemistry, Purdue University, 560 Oval Dr, West Lafayette, IN 47907 United States
AU: Shepson, P
EM: pshepson@purdue.edu
AF: Department of Chemistry, Purdue University, 560 Oval Dr, West Lafayette, IN 47907 United States
AU: Shepson, P
EM: pshepson@purdue.edu
AF: Department of Earth and Atmospheric Sciences, Purdue University, 550 Stadium Mall Dr, West Lafayette,
IN 47907 United States
AU: Rhodes, D
EM: drhodes@purdue.edu
AF: Department of Horticulture and Landscape Architecture, Purdue University, 625 Agriculture Mall Dr,
West Lafayette, IN 47907 United States
AB:
Changes in the global climate and atmosphere cause significant effects to the biosphere. Forests respond to these global
changes in various ways which all can affect their ability to store carbon, which in turn impacts climate change. Many
temperate latitude forests are nitrogen-limited. A current working hypothesis is that atmospheric nitrogen compounds that are
deposited to the canopy may be directly utilized by the plant as a nitrogen source. A significant fraction of atmospheric
reactive nitrogen that can be deposited is organic. Organic nitrogen deposition is not well characterized nor have the
ecological consequences been assessed. Our hypothesis is that organic nitrogen deposition to the canopy is significant, and
that that nitrogen is utilized by trees. Fumigation experiments were conducted with 14N and 15N-labeled organic nitrates
(focusing on 1-nitrooxy-3-methyl butane as a surrogate for isoprene nitrates) to determine if and how that nitrogen gets
incorporated into the leaves by detecting the 15N-labeled leaf amino acids. This research builds on work completed during
past summer intensives as part of the Program for Research on Oxidants: PHotochemistry, Emissions, and Transport (PROPHET),
and begins the next stage of research as part of the Biosphere Atmosphere Research \& Training program (BART) at the
University of Michigan Biological Station (UMBS). The overall goal of the new effort, the Biosphere Exchange of Atmospheric
Carbon and Odd Nitrogen (BEACON) program, is to evaluate the interactive roles of the atmosphere and forest in the coupling
of the carbon and nitrogen cycles.
DE: 0315 Biosphere/atmosphere interactions
DE: 0365 Troposphere--composition and chemistry
DE: 1615 Biogeochemical processes (4805)
SC: Atmospheric Sciences [A]
MN: 2003 Fall Meeting