HR: 0800h
AN: A21B-0847 [Abstracts]
TI: Implications of North American Boreal Fires on Air Quality and Composition in Nearby and Remote
Regions
AU: * Pfister, G G
EM: pfister@ucar.edu
AF: National Center for Atmospheric Research, 1850 Table Mesa Drive, Boulder, CO 80305
United States
AU: Emmons, L K
EM: emmons@ucar.edu
AF: National Center for Atmospheric Research, 1850 Table Mesa Drive, Boulder, CO 80305
United States
AU: Hess, P G
EM: hess@ucar.edu
AF: National Center for Atmospheric Research, 1850 Table Mesa Drive, Boulder, CO 80305
United States
AU: Lamarque, J
EM: lamar@ucar.edu
AF: National Center for Atmospheric Research, 1850 Table Mesa Drive, Boulder, CO 80305
United States
AU: Edwards, D P
EM: edwards@ucar.edu
AF: National Center for Atmospheric Research, 1850 Table Mesa Drive, Boulder, CO 80305
United States
AU: Thompson, A M
EM: anne@met.psu.edu
AF: Penn State University, 503 Walker Bldg, Univ Park, PA 16802
United States
AU: Wuebbles, D J
EM: wuebbles@atmos.uiuc.edu
AF: University of Illinois, 105 S. Gregory, Urbana, IL 61801
United States
AU: Herman, R L
EM: RL-Herman@wiu.edu
AF: Western Illinois University, 1 University Circle, Macomb, IL 61455
United States
AU: Owen, C R
EM: rcowen@mtu.edu
AF: Michigan Technological University, 1400 Townsend Drive, Houghton, MI 49931
United States
AU: Honrath, R
EM: reh@mtu.edu
AF: Michigan Technological University, 1400 Townsend Drive, Houghton, MI 49931
United States
AU: Val Martin, M
EM: mvalmart@mtu.edu
AF: Michigan Technological University, 1400 Townsend Drive, Houghton, MI 49931
United States
AU: Sachse, G W
EM: glen.w.sachse@nasa.gov
AF: NASA LaRC, MS 483, Hampton, VA 23681
United States
AU: Avery, M
EM: m.a.avery@larc.nasa.gov
AF: NASA LaRC, MS 483, Hampton, VA 23681
United States
AU: Randerson, J T
EM: jranders@uci.edu
AF: University of California, 3212 Croul Hall, Irvine, CA 92697
United States
AB:
During the summer of 2004, Alaska and Canada experienced intense wildfire episodes that emitted large amounts of pollutants
and aerosols into the atmosphere. We are using simulations with the global chemistry transport model MOZART to study the
impact of these emissions on air quality and composition over North America, the Northern Atlantic region, and Europe. The
emission inventory we apply for the Alaskan and Canadian wildfires in these simulations is based on a top-down approach using
MODIS fire counts, MOPITT CO observations, and the MOZART model. The model has been evaluated by comparison with a large
suite of observations such as data from ozone sondes, surface measurements of CO, ozone and nitrogen species, and aircraft
observations. The impact of the fires on the concentrations and distributions of the aforementioned trace species will be
discussed, including aspects related to air quality.
The mid- and lower tropospheric ozone load over North America for summer 2004 is about 7% higher in a simulation including
the Alaskan/Canadian wildfires compared to a reference simulation without fires in this region. During July 2004 we estimate
that, for about half the time, at least 30% of the ozone load in the lower and middle troposphere over Eastern Canada can be
attributed to chemical production from precursors emitted by the fires. Over Western Europe, we find contributions of 10%
and higher about one-third of the time. We are investigating the importance of the injection height of fire emissions on
atmospheric transport and chemistry, e.g. on the production of tropospheric ozone, and examine the effects of the
non-linearity in ozone chemistry. We further compare the radiative forcing of the fire induced increase in ozone
concentrations to the radiative forcing of greenhouse gases released by the fires such as CO2 and methane.
DE: 0365 Troposphere: composition and chemistry
DE: 0368 Troposphere: constituent transport and chemistry
DE: 0478 Pollution: urban, regional and global (0345, 4251)
DE: 1637 Regional climate change
SC: Atmospheric Sciences [A]
MN: Fall Meeting 2005