HR: 1340h
AN: GP13A-0016 [Abstracts]
TI: Low-temperature viscous magnetization of multidomain magnetite: evidence for disaccommodation
contribution
AU: * Muxworthy, A R
EM: adrian.muxworthy@gmail.com
AF: University of Southampton, NOC, European Way, Southampton, SO14 3ZH
United Kingdom
AU: Williams, W
EM: wyn.williams@ed.ac.uk
AF: University of Edinburgh, Geology, King's Buildings, West Mains Road, Edinburgh, EH9 3JW
United Kingdom
AB:
There are large gaps in our understanding of multidomain (MD) viscous behavior and MD remanence theory in general. For
example, Dunlop and ™zdemir (2000) have demonstrated that multidomain (MD) viscous remanent magnetization (VRM) acquired at
200 C in crushed and sized natural crystals of magnetite persists on thermal demagnetization up to the Curie temperature,
that is, there is a MD VRM component which is metastable. This goes against the classic MD theory of N‚el which predicts that
domain walls which move at low-temperatures in the earth's field, are easily re-organized by small increases in
temperatures. That is, theory predicts that any VRM acquired by domain walls at 200 C will not persist to the Curie
temperature.
Recent viscosity experiments at temperatures above room-temperature have revealed that MD viscosity has a complex dependency
on the magnetization state, dislocation density, disaccommodation, stoichiometry and thermal history. In particular the
contribution of disaccommodation to viscosity has been difficult to isolate. Below room-temperature, disaccommodation
displays a large increase, therefore by measuring viscosity below room temperature, then its contribution can be more readily
assessed.
Low-temperature viscous acquisition and decay measurements above and below the Verwey transition have been measured for a
selection of natural and synthetic multidomain magnetite samples. A strong correlation between the viscosity spectra and
published disaccommodation spectra was found, where disaccommodation reflects electron mobility. Assuming the viscosity is
controlled by identical mechanisms as disaccommodation, the reduction in electron mobility below the Verwey transition is
found to significantly increase viscous acquisition and decay rates over the time scales measured (1-3000 seconds). Although
strongly affecting the viscosity, disaccommodation processes do not appear to control the rate of change of viscosity with
time, i.e., the viscosity curvature. It is suggested that the curvature is controlled by the shape of relaxation-time
distributions, which is approximately the same for all the magnetite samples studied. In addition, the acquisition and decay
curvature parameters mirror each other when plotted as a function of temperature, inferring that at any given temperature the
acquisition and decay processes are identical.
DE: 1540 Rock and mineral magnetism
SC: Geomagnetism and Paleomagnetism [GP]
MN: Fall Meeting 2005