HR: 1340h
AN: H33A-1380 [Abstracts]
TI: Pore-Scale Acoustic Effects on Colloid Interactions at Solid/Liquid Interfaces under Varying
Physicochemical Conditions
AU: * Roberts, P M
EM: proberts@lanl.gov
AF: Los Alamos National Laboratory, PO Box 1663
MS-D443, Los Alamos, NM 87545
United States
AB:
Acoustic energy can produce enhanced attachment and/or detachment of colloids at solid/liquid interfaces. This, in turn, can
cause changes in colloid and fluid transport through porous media that depend strongly on the physical and chemical
properties of the porous matrix, the fluid contained in the matrix pore space, and the colloids suspended in the fluid.
Accumulation or release of colloids can alter the permeability of the porous medium. This can cause either good or bad
effects on porous fluid-flow behavior in the Earth and geomaterials. Prior experiments using a microscopic, video
image-processing system focused on a glass flow-visualization cell indicated that 0.5 to 5 MHz acoustic energy can induce
attachment and detachment of sub-micron-size polystyrene microspheres at solid/liquid interfaces, using 0.1 M NaCl solution
as the suspending fluid. New experiments were performed under differing initial conditions of ionic strength and solid
surface properties, and at different acoustic frequencies. Initial results of these microscopic experiments will be
presented. Other prior experiments showed that 50 Hz mechanical stress oscillations can mobilize trapped in-situ colloids in
centimeter-size sandstone cores. A unique core-holder apparatus that mechanically strains 2.54-cm-diameter porous rock
samples during constant-rate fluid flow was used for those experiments. New experiments were performed by injecting into
clean core samples the same polystyrene microsphere suspensions used in the microscopic visualization experiments.
Microsphere trapping in the core was induced by using a high ionic strength suspending solution. The core was then flushed
with de-ionized water. This caused rapid release of the majority of trapped microspheres. Stress stimulation at 26 Hz caused
additional releases of the remaining trapped microspheres at a rate approximately 4 times higher than the average background
rate during water flow alone. Results of several core-scale experiments run over a range of ionic strengths will be
presented.
DE: 1835 Hydrogeophysics
DE: 1859 Rocks: physical properties
DE: 1899 General or miscellaneous
DE: 4499 General or miscellaneous
SC: Hydrology [H]
MN: Fall Meeting 2005