HR: 0800h
AN: P21A-0126 [Abstracts]
TI: Distinguishing Na, K, and H3O+ Jarosite and Alunite on Mars using VNIR, Emittance and M”ssbauer
Spectroscopy on the MER and Mars Express/OMEGA Missions
AU: * Bishop, J L
EM: jbishop@arc.nasa.gov
AF: SETI Institute & NASA-Ames Research Center, 515 N. Whisman Rd, Mountain View, CA 94560
AU: Rothstein, Y
P21A-0126
AF: Mount Holyoke College, 50 College St., South Hadley, MA 01075
AU: Dyar, M D
P21A-0126
AF: Mount Holyoke College, 50 College St., South Hadley, MA 01075
AU: Lane, M D
P21A-0126
AF: Planetary Science Institute, 620 North Sixth Avenue, Tucson, AZ 85705
AU: Klima, R L
P21A-0126
AF: Brown University, Department of Geological Sciences, Providence, RI 02912
AU: Brophy, G P
P21A-0126
AF: Amherst College, Department of Geology, Amherst, MA 01002
AB:
Jarosite has been identified in layered outcrops in Meridiani by the MER Mossbauer spectrometer [Klingelh”fer, et al., 2004]
and may be present elsewhere on Mars. We are studying VNIR, emittance and M”ssbauer spectroscopy of a suite of synthetic and
natural samples of jarosite and alunite from the Brophy collection [e.g. Brophy and Sheridan, 1965]. The characteristic NIR
overtones and combination bands in this group differ not only depending on the trivalent cation (e.g. Al for alunite and Fe
for jarosite), but also depending on the type of monovalent cation (typically K, Na and/or H3O).
The VNIR spectrum of K-jarosite exhibits an OH stretching band at 1.47 um, an OH stretch + 2 bend combination doublet at
1.849 and 1.864 um, plus an OH stretch + bend combination triplet at 2.215, 2.265, and 2.300 um and additional OH and SO4
combination features near 2.40, 2.46, 2.50, 2.60 and 2.62 um. H3O- and Na-jarosite spectra exhibit broader features and the
doublet is less resolvable. The spectrum of Na-jarosite contains a band at 1.48 um, a broad asymmetric band near 1.85 um and
a triplet near 2.235, 2.275, and 2.310 um, plus additional features near 2.42, 2.47, 2.52, 2.62 and 2.64 um. Band assignments
for jarosite and alunite spectra are from Bishop and Murad [2005]. We are in the process of comparing these spectra with the
mid-IR and Mossbauer spectra of this jarosite group sample suite in order to perform coordinated analyses for this sulfate
group on Mars using the MER and Mars Express datasets.
References:
Bishop, J. L., and E. Murad (2005), The visible and infrared spectral properties of jarosite and alunite, Am. Miner., 90,
1100-1107.
Brophy, G. P., and M. F. Sheridan (1965), Sulfate studies IV: The jarosite-natrojarosite-hydronium jarosite solid solution
series, Am. Miner., 50, 1595-1607.
Klingelh”fer, G., et al. (2004), Jarosite and hematite at Meridiani Planum from Opportunity's M”ssbauer spectrometer,
Science, 306, 1740-1745.
DE: 3929 NMR, Mossbauer spectroscopy, and other magnetic techniques
DE: 3934 Optical, infrared, and Raman spectroscopy
DE: 5464 Remote sensing
DE: 6225 Mars
SC: Planetary Sciences [P]
MN: Fall Meeting 2005