HR: 0800h
AN: H51D-1172 [Abstracts]
TI: Separation in storm-event trajectories of DOC and nitrate concentrations with seasons
AU: Graham, J
EM: jmgraham888@yahoo.com
AF: SUNY College at Buffalo, 1300 Elmwood Avenue
Great Lakes Center HC 215, Buffalo, NY 14222
United States
AU: * Inamdar, S
EM: inamdasp@buffalostate.edu
AF: SUNY College at Buffalo, 1300 Elmwood Avenue
Great Lakes Center HC 215, Buffalo, NY 14222
United States
AU: Mitchell, M
EM: mitchell@mailbox.syr.edu
AF: SUNY-ESF, 1 Forestry Drive, Syracuse, NY 14210
United States
AU: Tuk, J
EM: jmtuk27@yahoo.com
AF: SUNY College at Buffalo, 1300 Elmwood Avenue
Great Lakes Center HC 215, Buffalo, NY 14222
United States
AB:
The temporal evolution of DOC and nitrate concentrations during storm events and the flow paths responsible for their release
have received considerable attention. Some researchers observed DOC and nitrate peaks on the hydrograph rising limb and
attributed it to "flushing". Flushing was defined as the release of solutes from near-surface soil layers associated with a
rising water table. In contrast, others found a nitrate peak on the rising limb and a delayed DOC peak at or after discharge
peak. In this case, the early nitrate peak was attributed to "displacement" of groundwater into the stream and the DOC peak
was attributed to flushing. We studied the temporal patterns of storm-event DOC and nitrate for more than 20 storm events
over a year in a watershed in Western New York, USA. Storm event sampling was conducted across four partly nested catchments
- 696 (s1), 3.4 (s2), 1.6 (s3) and 1.9 (s5) ha. The four watersheds contained varying proportions of hillslope and
valley-bottom saturated areas. Early spring rainfall events showed very similar nitrate and DOC trajectories with a peak in
concentration at or after the discharge peak. Riparian groundwater elevations showed peak water tables coinciding with
solute peaks suggesting flushing of both DOC and nitrate from the catchment. For summer and fall events however, there was a
clear separation between the DOC and nitrate trajectories. Nitrate was at its highest early on in the storm event and then
followed a dilution trajectory as the event proceeded. DOC concentrations increased through the event (as nitrate dropped)
with a peak in concentration just after discharge peak. This seasonal shift in DOC and nitrate trajectories was observed
across catchment scales. These observations show that both flushing and displacement mechanisms could occur in a watershed
and their expression is regulated by the availability of the solutes in the soil profile. DOC concentrations were found to
be high in upper soil layers across all seasons, but nitrate build-up in the upper soil layers was limited to the dormant
period before spring onset. We hypothesize that the temporal expression of solutes (especially DOC) is regulated by the total
extent of the saturation in the watershed, the areal distribution of the saturated areas and their connectedness, and the
seasonally regulated availability of the solutes. These hypotheses are currently being evaluated by comparing the temporal
expressions across catchment scales.
UR: http://www.buffalostate.edu/orgs/glc/gowanda/overview.htm
DE: 1860 Runoff and streamflow
DE: 1871 Surface water quality
SC: Hydrology [H]
MN: 2004 AGU Fall Meeting