HR: 1340h
AN: MR23A-0193 [Abstracts]
TI: MgO: \textit{ab initio} equation of state and its dislocation
properties from molecular dynamics simulations*
AU: Swift, D
AF: Physics Division, Los Alamos National Laboratory, Los Alamos, NM 87545
United States
AU: * Luo, S
EM: sluo@lanl.gov
AF: Physics Division, Los Alamos National Laboratory, Los Alamos, NM 87545
United States
AU: Strachan, A
AF: Theoretical Division, Los Alamos National Laboratory, Los Alamos, NM 87545
United States
AU: Huang, H
AF: Materials and Process Simulation Center, California Institute of Technology, Pasadena, CA 91125
United States
AU: Mulford, R
AF: NMT Division, Los Alamos National Laboratory, Los Alamos, NM 87545
AU: Drummond, N
AF: Department of Physics and Astronomy, University of Edinburg, Edinburg, EH9 3JZ
United Kingdom
AU: Ackland, G
AF: Department of Physics and Astronomy, University of Edinburg, Edinburg, EH9 3JZ
United Kingdom
AU: Goddard, W
AF: Materials and Process Simulation Center, California Institute of Technology, Pasadena, CA 91125
United States
AB:
The equation of state (EOS) of MgO, and its
dislocation properties were investigated using
{\it ab initio} quantum-mechanics techniques and
classical molecular dynamics (MD) with a Morse-stretch
charge-equilibrium potential, respectively.
The thermodynamically complete
{\it ab initio} EOS was demonstrated to be consistent with the isotherm,
thermal expansivity, heat capacity and melting curve measured in
static experiments, and reproduced density and temperature measurements
under shock wave loading of bulk and porous periclase. The melting locus
of MgO, relevant to the Earth's lower mantle pressures, was predicted to be accessible
by shock wave loading of porous periclase.
Preliminary MD simulations of dislocations in MgO
indicated qualitative similarity to measurements of the temperature--stress
curve, and revealed a qualitative understanding of the
mechanism behind non-conservative motion of edge dislocations in MgO.
*Work partly performed under the auspices of the US Department of Energy
under contract No. W-7405-ENG-36.
DE: 3909 Elasticity and anelasticity
DE: 3919 Equations of state
DE: 3924 High-pressure behavior
DE: 3944 Shock wave experiments
SC: Mineral and Rock Physics [MR]
MN: 2004 AGU Fall Meeting