HR: 1340h
AN: A33E-1644 [Abstracts]
TI: Physical and Radiative Properties of Aerosol Particles in the Caribbean: Influence of African Dust and Soufriere Volcanic Ash
AU: * Villanueva-Birriel, C M
EM: cecillem28@gmail.com
AF: Department of Physics, University of Puerto Rico, Rio Piedras, PO BOX 23343, San Juan,
PR 00931-3343, Puerto Rico
AU: * Villanueva-Birriel, C M
EM: cecillem28@gmail.com
AF: Institute for Tropical Ecosystem Studies (ITES), University of Puerto Rico, Rio Piedras, PO
Box 21910, San Juan, PR 00931-1910, Puerto Rico
AU: Mayol-Bracero, O L
EM: omayol@adam.uprr.pr
AF: Institute for Tropical Ecosystem Studies (ITES), University of Puerto Rico, Rio Piedras, PO
Box 21910, San Juan, PR 00931-1910, Puerto Rico
AU: Sheridan, P
EM: Patrick.Sheridan@noaa.gov
AF: NOAA Earth System Research Laboratory, Global Monitoring Division/GMD-1
325 Broadway, Boulder, CO 80305, United States
AU: Ogren, J A
EM: John.A.Ogren@noaa.gov
AF: NOAA Earth System Research Laboratory, Global Monitoring Division/GMD-1
325 Broadway, Boulder, CO 80305, United States
AB:
Atmospheric particles such as dust and volcanic ash have the potential of influencing the
earth's
radiative budget directly by scattering or absorbing solar radiation in the atmosphere and indirectly by affecting
cloud condensation nuclei (CCN) concentrations and, therefore, cloud albedo. The radiatively-important
properties of atmospheric particles are determined at the most fundamental level by their chemical composition
and size distributions; therefore, the importance of studying the chemical, physical, and optical aerosol
properties.
Over the summer months, the island of Puerto Rico receives African dust incursions that reduce visibility and
have an impact on public health, ecosystem, and climate. Visibility is also negatively affected when the island
receives south-east winds and the Soufriere volcano (Montserrat Island) has been active. Here we present
preliminary results of measurements performed during 2006 and 2007 at Cape San Juan, a ground-based
station located at the northeastern tip of Puerto Rico. The cases investigated showed three possible types of air
masses: clean (C), with African Dust (AD), and with volcanic ash (VA) from the Soufriere. We used a
condensation particle counter to determine the particle number concentration, a sunphotometer (part of the
AERONET) to determine volume size distributions and aerosol optical thickness (AOT), a 3-wavelength
nephelometer to determine the scattering coefficients, and a 3-wavelength particle/soot absorption photometer
(PSAP) for the absorption coefficients. The particle number concentrations were higher for AD and VA periods (up
to about 700 cm-3 on average for both cases) in contrast to ~400 cm-3 for the C period. Volume size distributions
showed bimodal distributions for the three cases with a greater influence of the coarse fraction for the C and VA
periods and an increase in the fine particles for the AD period. The total scattering coefficient showed higher
values for the AD (30 Mm-1) and the VA (26 Mm-1) cases than for the C case (11 Mm-1). The highest AOT values
(at 500 nm) were observed for the AD and VA cases (up to ~0.35 and 0.3, respectively). C samples had much
lower AOT values (~ 0.07). Our preliminary results clearly showed an impact of African dust and volcanic ash on
the physical and radiative properties of aerosol particles. Results on the chemical composition of particles
representative of the three cases will also be presented at the meeting.
DE: 0305 Aerosols and particles (0345, 4801, 4906)
SC: Atmospheric Sciences [A]
MN: 2007 Fall Meeting