HR: 16:30h
AN: A34A-03 [Abstracts]
TI: The Impact of Aerosol Sources and Aging on CCN Formation in the Houston-Galveston-Gulf of Mexico Region
AU: * Quinn, P
EM: patricia.k.quinn@noaa.gov
AF: NOAA PMEL, 7600 Sand Point Way NE, Seattle, WA 98115,
AU: Bates, T
EM: tim.bates@noaa.gov
AF: NOAA PMEL, 7600 Sand Point Way NE, Seattle, WA 98115,
AU: Coffman, D
EM: derek.coffman@noaa.gov
AF: NOAA PMEL, 7600 Sand Point Way NE, Seattle, WA 98115,
AU: Covert, D
EM: dcovert@u.washington.edu
AF: University of Washington, 4909 25th Ave NE, Seattle, WA 98105,
AB:
The impact of anthropogenic aerosol on cloud properties, cloud lifetime, and precipitation processes is one of the
largest uncertainties in our current understanding of climate change. Aerosols affect cloud properties by serving
as cloud condensation nuclei (CCN) thereby leading to the formation of cloud droplets. The process of cloud drop
activation is a function of both the size and chemistry of the aerosol particles which, in turn, depend on the source
of the aerosol and transformations that occur downwind. In situ field measurements that can lead to an improved
understanding of the process of cloud drop formation and simplifying parameterizations for improving the
accuracy of climate models are highly desirable. During the Gulf of Mexico Atmospheric Composition and Climate
Study (GoMACCS), the NOAA RV Ronald H. Brown encountered a wide variety of aerosol types ranging from
marine near the Florida panhandle to urban and industrial in the Houston-Galveston area. These varied sources
provided an opportunity to investigate the role of aerosol sources, aging, chemistry, and size in the activation of
particles to form cloud droplets.
Here, we use the correlation between variability in critical diameter for activation (determined empirically from
measured CCN concentrations and the number size distribution) and aerosol composition to quantify the impact
of composition on particle activation. Variability in aerosol composition is parameterized by the mass fraction of
Hydrocarbon-like Organic Aerosol (HOA) for particle diameters less than 200 nm (vacuum aerodynamic). The
HOA mass fraction in this size range is lowest for marine aerosol and higher for aerosol impacted by
anthropogenic emissions. Combining all data collected at 0.44 percent supersaturation (SS) reveals that
composition (defined in this way) explains 40 percent of the variance in the critical diameter. As expected, the
dependence of activation on composition is strongest at lower SS. At the same time, correlations between HOA
mass fraction and aerosol mean diameter show that these two parameters are essentially independent of one
another for this data set. We conclude that, based on the variability of the HOA mass fraction observed during
GoMACCS, composition plays a dominant role in determining the fraction of particles that are activated to form
cloud droplets.
Using Kohler theory, we estimate the error that results in calculated CCN concentrations if the organic fraction of
the aerosol is neglected (i.e., a fully soluble composition of ammonium sulfate is assumed) for the range of
organic mass fractions and mean diameters observed during GoMACCS. We then relate this error to the source
and age of the aerosol. At 0.22 and 0.44 percent SS, the error is considerable for anthropogenic aerosol sampled
near the source region as this aerosol has, on average, a high POM mass fraction and smaller particle mean
diameter. The error is lower for more aged aerosol as it has a lower POM mass fraction and larger mean particle
diameter. Hence, the percent error in calculated CCN concentration is expected to be larger for younger, organic-
rich aerosol and smaller for aged, sulfate rich aerosol and for marine aerosol. We extend this analysis to
continental and marine data sets recently reported by Dusek et al. [Science, 312, 1375, 2006] and Hudson
[Geophys. Res., Lett., 34, L08801, 2007].
DE: 0305 Aerosols and particles (0345, 4801, 4906)
DE: 0320 Cloud physics and chemistry
DE: 0345 Pollution: urban and regional (0305, 0478, 4251)
SC: Atmospheric Sciences [A]
MN: 2007 Fall Meeting