HR: 16:40h
AN: A44A-02 INVITED     [Abstracts]
TI: Ozone Air Quality and Radiative Forcing Consequences of Changes in Ozone Precursor Emissions
AU: * West, J
EM: jwest@princeton.edu
AF: Atmospheric & Oceanic Sciences Program, Princeton University, Sayre Hall, Princeton, NJ 08544, United States
AU: * West, J
EM: jwest@princeton.edu
AF: Woodrow Wilson School of Public & International Affairs, Princeton University, Robertson Hall, Princeton, NJ 08544, United States
AU: * West, J
EM: jwest@princeton.edu
AF: Department of Environmental Sciences and Engineering, University of North Carolina, Chapel Hill, CB #7431, Rosenau Hall, Chapel Hill, NC 27599, United States
AU: Fiore, A M
EM: arlene.fiore@noaa.gov
AF: NOAA Geophysical Fluid Dynamics Laboratory, 201 Forrestal Road, Princeton, NJ 08540, United States
AU: Naik, V
EM: vnaik@princeton.edu
AF: Woodrow Wilson School of Public & International Affairs, Princeton University, Robertson Hall, Princeton, NJ 08544, United States
AU: Horowitz, L W
EM: larry.horowitz@noaa.gov
AF: NOAA Geophysical Fluid Dynamics Laboratory, 201 Forrestal Road, Princeton, NJ 08540, United States
AU: Schwarzkopf, M
EM: dan.schwarzkopf@noaa.gov
AF: NOAA Geophysical Fluid Dynamics Laboratory, 201 Forrestal Road, Princeton, NJ 08540, United States
AU: Mauzerall, D L
EM: mauzeral@princeton.edu
AF: Woodrow Wilson School of Public & International Affairs, Princeton University, Robertson Hall, Princeton, NJ 08544, United States
AU: Mauzerall, D L
EM: mauzeral@princeton.edu
AF: Department of Geosciences, Guyot Hall, Princeton, NJ 08544, United States
AB: Changes in emissions of ozone (O3) precursors affect both air quality and climate. We first examine the sensitivity of surface O3 concentrations (O3srf) and net radiative forcing of climate (RFnet) to reductions in emissions of four precursors - nitrogen oxides (NOx), non-methane volatile organic compounds, carbon monoxide, and methane (CH4). We show that long-term CH4-induced changes in O3, known to be important for climate, are also relevant for air quality; for example, NOx reductions increase CH4, causing a long-term O3 increase that partially counteracts the direct O3 decrease. Second, we assess the radiative forcing resulting from actions to improve O3 air quality by calculating the ratio of ΔRFnet to changes in metrics of O3srf. Decreases in CH4 emissions cause the greatest RFnet decrease per unit reduction in O3srf, while NOx reductions increase RFnet. Of the available means to improve O3 air quality, therefore, CH4 abatement best reduces climate forcing.
DE: 0365 Troposphere: composition and chemistry
DE: 0368 Troposphere: constituent transport and chemistry
DE: 1610 Atmosphere (0315, 0325)
DE: 3305 Climate change and variability (1616, 1635, 3309, 4215, 4513)
SC: Atmospheric Sciences [A]
MN: 2007 Joint Assembly